We gratefully acknowledge support from
the Simons Foundation and member institutions.
Full-text links:

Download:

Current browse context:

cond-mat.str-el

Change to browse by:

References & Citations

Bookmark

(what is this?)
CiteULike logo BibSonomy logo Mendeley logo del.icio.us logo Digg logo Reddit logo

Condensed Matter > Strongly Correlated Electrons

Title: Gapless quantum spin liquid in the triangular system Sr$_{3}$CuSb$_{2}$O$_{9}$

Abstract: We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated by Sb planes. Muon spin relaxation ($\mu$SR) measurements show that the $S = \frac{1}{2}$ moments at the magnetically active Cu sites remain dynamic down to 65 mK in spite of a large antiferromagnetic exchange scale evidenced by a large Curie-Weiss temperature $\theta_{\mathrm{cw}} \simeq $ -143 K as extracted from the bulk susceptibility. Specific heat measurements also show no sign of long-range order down to 0.35 K. The magnetic specific heat ($\mathit{C}$$_{\mathrm{m}}$) below 5 K reveals a $\mathit{C}$$_{\mathrm{m}}$ $=$ $\gamma T$ + $\alpha T$$^{2}$ behavior. The significant $T$$^{2}$ contribution to the magnetic specific heat invites a phenomenology in terms of the so-called Dirac spinon excitations with a linear dispersion. From the low-$T$ specific heat data, we estimate the dominant exchange scale to be $\sim $ 36 K using a Dirac spin liquid ansatz which is not far from the values inferred from microscopic density functional theory calculations ($\sim $ 45 K) as well as high-temperature susceptibility analysis ($\sim$ 70 K). The linear specific heat coefficient is about 18 mJ/mol-K$^2$ which is somewhat larger than for typical Fermi liquids.
Comments: 16 pages, 21 figures, including supplementary material. A $S = \frac{1}{2}$ Dirac spin liquid scenario has been put forward to explain the field-dependent specific heat data. Comments are welcome
Subjects: Strongly Correlated Electrons (cond-mat.str-el)
Journal reference: Phys. Rev. Lett. 125, 267202 (2020)
DOI: 10.1103/PhysRevLett.125.267202
Cite as: arXiv:2012.01239 [cond-mat.str-el]
  (or arXiv:2012.01239v3 [cond-mat.str-el] for this version)

Submission history

From: Susanta Kundu [view email]
[v1] Wed, 2 Dec 2020 14:31:19 GMT (1555kb,D)
[v2] Mon, 14 Dec 2020 12:58:38 GMT (3052kb,D)
[v3] Mon, 28 Dec 2020 15:48:32 GMT (3053kb,D)

Link back to: arXiv, form interface, contact.