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Condensed Matter > Mesoscale and Nanoscale Physics

Title: Photoluminescence imaging of single photon emitters within nanoscale strain profiles in monolayer WSe$_2$

Abstract: Local deformation of atomically thin van der Waals materials provides a powerful approach to create site-controlled chip-compatible single-photon emitters (SPEs). However, the microscopic mechanisms underlying the formation of such strain-induced SPEs are still not fully clear, which hinders further efforts in their deterministic integration with nanophotonic structures for developing practical on-chip sources of quantum light. Here we investigate SPEs with single-photon purity up to 98% created in monolayer WSe$_2$ via nanoindentation. Using photoluminescence imaging in combination with atomic force microscopy, we locate single-photon emitting sites on a deep sub-wavelength spatial scale and reconstruct the details of the surrounding local strain potential. The obtained results suggest that the origin of the observed single-photon emission is likely related to strain-induced spectral shift of dark excitonic states and their hybridization with localized states of individual defects.
Comments: 8 pages, 4 figures
Subjects: Mesoscale and Nanoscale Physics (cond-mat.mes-hall); Quantum Physics (quant-ph)
DOI: 10.1038/s41467-023-41292-9
Cite as: arXiv:2301.09478 [cond-mat.mes-hall]
  (or arXiv:2301.09478v1 [cond-mat.mes-hall] for this version)

Submission history

From: Artem Abramov [view email]
[v1] Mon, 23 Jan 2023 15:21:28 GMT (8883kb,D)

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