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Condensed Matter > Strongly Correlated Electrons

Title: Easy-plane multi-$\mathbf{q}$ magnetic ground state of Na$_3$Co$_2$SbO$_6$

Abstract: Na$_3$Co$_2$SbO$_6$ is a potential Kitaev magnet with a monoclinic layered crystal structure. Recent investigations of the $C_3$-symmetric sister compound Na$_2$Co$_2$TeO$_6$ have uncovered a unique triple-$\mathbf{q}$ magnetic ground state, as opposed to a single-$\mathbf{q}$ (zigzag) one, prompting us to examine the influence of the reduced structural symmetry of Na$_3$Co$_2$SbO$_6$ on its ground state. Neutron diffraction data obtained on a twin-free crystal reveal that the ground state remains a multi-$\mathbf{q}$ state, despite the system's strong in-plane anisotropy. This robustness of multi-$\mathbf{q}$ orders suggests that they are driven by a common mechanism in the honeycomb cobaltates, such as higher-order magnetic interactions. Spin-polarized neutron diffraction results show that the ordered moments are entirely in-plane, with each staggered component orthogonal to the propagating wave vector. The inferred ground state favors a so-called XXZ easy-plane anisotropic starting point for the microscopic model over a Kitaev one, and features unequal ordered moments reduced by strong quantum fluctuations.
Comments: 4 pages, 4 figures, plus Supplemental Material
Subjects: Strongly Correlated Electrons (cond-mat.str-el)
Journal reference: Physical Review B 109, L060410 (2024)
DOI: 10.1103/PhysRevB.109.L060410
Cite as: arXiv:2306.07175 [cond-mat.str-el]
  (or arXiv:2306.07175v1 [cond-mat.str-el] for this version)

Submission history

From: Yuan Li [view email]
[v1] Mon, 12 Jun 2023 15:14:20 GMT (6406kb,D)

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