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Condensed Matter > Strongly Correlated Electrons

Title: High thermoelectric power factor through topological flat bands

Abstract: Thermoelectric (TE) materials are useful for applications such as waste heat harvesting or efficient and targeted cooling. While various strategies towards superior thermoelectrics through a reduction of the lattice thermal conductivity have been developed, a path to enhance the power factor is pressing. Here, we report large power factors up to 5 mW m$^{-1}$ K$^{-2}$ at room temperature in the kagome metal Ni$_3$In$_{1-x}$Sn$_x$. This system is predicted to feature almost dispersionless flat bands in conjunction with highly dispersive Dirac-like bands in its electronic structure around the Fermi energy $E_\text{F}$ [L. Ye et al., Nature Physics 1-5 (2024)]. Within this study, we experimentally and theoretically showcase that tuning this flat band precisely below $E_\text{F}$ by chemical doping $x$ boosts the Seebeck coefficient and power factor, as highly mobile charge carriers scatter into the flat-band states. Our work demonstrates the prospect of engineering extremely flat and highly dispersive bands towards the Fermi energy in kagome metals and introduces topological flat bands as a novel tuning knob for thermoelectrics.
Subjects: Strongly Correlated Electrons (cond-mat.str-el)
Cite as: arXiv:2404.08067 [cond-mat.str-el]
  (or arXiv:2404.08067v1 [cond-mat.str-el] for this version)

Submission history

From: Fabian Garmroudi [view email]
[v1] Thu, 11 Apr 2024 18:13:20 GMT (1308kb,D)

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