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Condensed Matter > Mesoscale and Nanoscale Physics

Title: Observation of Floquet states in graphene

Authors: Marco Merboldt (1), Michael Schüler (2 and 3), David Schmitt (1), Jan Philipp Bange (1), Wiebke Bennecke (1), Karun Gadge (4), Klaus Pierz (5), Hans Werner Schumacher (5), Davood Momeni (5), Daniel Steil (1), Salvatore R. Manmana (4), Michael Sentef (6 and 7), Marcel Reutzel (1), Stefan Mathias (1 and 8) ((1) I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, (2) Laboratory for Materials Simulations, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland, (3) Department of Physics, University of Fribourg, CH-1700 Fribourg, Switzerland, (4) Institut für Theoretische Physik, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, (5) Physikalisch-Technische Bundesanstalt, Bundesallee 100, 38116 Braunschweig, Germany, (6) Institute for Theoretical Physics and Bremen Center for Computational Materials Science, University of Bremen, 28359 Bremen, Germany, (7) Max Planck Institute for the Structure and Dynamics of Matter, Center for Free-Electron Laser Science (CFEL), Luruper Chaussee 149, 22761 Hamburg, Germany, (8) International Center for Advanced Studies of Energy Conversion (ICASEC), University of Göttingen, Göttingen, Germany)
Abstract: Recent advances in the field of condensed-matter physics have unlocked the potential to realize and control emergent material phases that do not exist in thermal equilibrium. One of the most promising concepts in this regard is Floquet engineering, the coherent dressing of matter via time-periodic perturbations. However, the broad applicability of Floquet engineering to quantum materials is still unclear. For the paradigmatic case of monolayer graphene, the theoretically predicted Floquet-induced effects, despite a seminal report of the light-induced anomalous Hall effect, have been put into question. Here, we overcome this problem by using electronic structure measurements to provide direct experimental evidence of Floquet engineering in graphene. We report light-matter-dressed Dirac bands by measuring the contribution of Floquet sidebands, Volkov sidebands, and their quantum path interference to graphene's photoemission spectral function. Our results finally demonstrate that Floquet engineering in graphene is possible, paving the way for the experimental realization of the many theoretical proposals on Floquet-engineered band structures and topological phases.
Comments: 4 main figures, 3 extended figures
Subjects: Mesoscale and Nanoscale Physics (cond-mat.mes-hall)
Cite as: arXiv:2404.12791 [cond-mat.mes-hall]
  (or arXiv:2404.12791v1 [cond-mat.mes-hall] for this version)

Submission history

From: Marcel Reutzel [view email]
[v1] Fri, 19 Apr 2024 11:05:53 GMT (2929kb,D)

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