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Condensed Matter > Disordered Systems and Neural Networks

Title: Experimental evidence for the $ω^4$ tail of the nonphononic spectra of glasses

Abstract: It is now established that glasses feature low-frequency, nonphononic excitations, in addition to phonons that follow Debye's vibrational density of state (VDoS). Extensive computer studies demonstrated that these nonphononic, glassy excitations follow a universal non-Debye VDoS ${\cal D}_{\rm G}(\omega)\!\sim\!\omega^4$, at low frequencies $\omega$. Yet, due to intrinsic difficulties in disentangling ${\cal D}_{\rm G}(\omega)$ from the total VDoS ${\cal D}(\omega)$, which is experimentally accessible through various scattering techniques, the $\omega^4$ tail of ${\cal D}_{\rm G}(\omega)$ lacked direct experimental support. We develop a procedure to extract ${\cal D}_{\rm G}(\omega)$ from the measured ${\cal D}(\omega)$, based on recent advances in understanding low-frequency excitations in glasses, and apply it to available datasets for diverse glasses. The resulting analysis shows that the $\omega^4$ tail of the nonphononic vibrational spectra of glasses is nontrivially consistent with a broad range of experimental observations. It also further supports that ${\cal D}_{\rm G}(\omega)$ makes an additive contribution to ${\cal D}(\omega)$.
Comments: 5 pages, 3 figures + Supplemental materials + Bibliographical list; see related work at: this https URL
Subjects: Disordered Systems and Neural Networks (cond-mat.dis-nn); Materials Science (cond-mat.mtrl-sci); Soft Condensed Matter (cond-mat.soft)
Cite as: arXiv:2404.16996 [cond-mat.dis-nn]
  (or arXiv:2404.16996v1 [cond-mat.dis-nn] for this version)

Submission history

From: Eran Bouchbinder [view email]
[v1] Thu, 25 Apr 2024 19:33:08 GMT (713kb,D)

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