Title: Calculation of the biquadratic spin interactions based on the spin cluster expansion for \textit{ab initio} tight-binding models

Abstract: We devise a calculation scheme for \textit{ab initio} tight-binding Hamiltonians to evaluate the biquadratic spin interaction. This scheme employs the spin cluster expansion with the disordered local moment method and was originally developed within the Korringa-Kohn-Rostoker theory. By applying it to the two-orbital Hubbard model, we show that the evaluated biquadratic interactions agree well with those in the effective quantum spin model derived for the limit of strong correlation. This result suggests the broad applicability of the method to various magnets with large local moments. We then apply it to the \textit{ab initio} tight-binding models for bcc Fe and fcc Ni and obtain consistent results with previous studies. The present scheme offers a convenient \textit{ab initio} tool for understanding or predicting magnetic properties arising from the biquadratic interaction.