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Condensed Matter > Materials Science

Title: Deep-ultraviolet transparent conducting SrSnO3 via heterostructure design

Abstract: Exploration and advancements in ultra-wide bandgap (UWBG) semiconductors are pivotal for next-generation high-power electronics and deep-ultraviolet (DUV) optoelectronics. A critical challenge lies in finding a semiconductor that is highly transparent to DUV wavelengths yet conductive with high mobility at room temperature. Here, we achieved both high transparency and high conductivity by employing a thin heterostructure design. The heterostructure facilitated high conductivity by screening phonons using free carriers, while the atomically thin films ensured high transparency. We utilized a heterostructure comprising SrSnO3/La:SrSnO3/GdScO3 (110) and applied electrostatic gating to effectively separate electrons from their dopant atoms. This led to a modulation of carrier density from 1018 cm-3 to 1020 cm-3, with room temperature mobilities ranging from 40 to 140 cm2V-1s-1. The phonon-limited mobility, calculated from first principles, closely matched experimental results, suggesting that room-temperature mobility could be further increased with higher electron density. Additionally, the sample exhibited 85% optical transparency at a 300 nm wavelength. These findings highlight the potential of heterostructure design for transparent UWBG semiconductor applications, especially in deep-ultraviolet regime.
Comments: 32 pages
Subjects: Materials Science (cond-mat.mtrl-sci)
Cite as: arXiv:2405.08915 [cond-mat.mtrl-sci]
  (or arXiv:2405.08915v1 [cond-mat.mtrl-sci] for this version)

Submission history

From: Bharat Jalan [view email]
[v1] Tue, 14 May 2024 19:09:51 GMT (6479kb)

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