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Condensed Matter > Strongly Correlated Electrons

Title: Signatures of ultrafast reversal of excitonic order in Ta$_2$NiSe$_5$

Abstract: In the presence of electron-phonon coupling, an excitonic insulator harbors two degenerate ground states described by an Ising-type order parameter. Starting from a microscopic Hamiltonian, we derive the equations of motion for the Ising order parameter in the phonon coupled excitonic insulator Ta$_2$NiSe$_5$ and show that it can be controllably reversed on ultrashort timescales using appropriate laser pulse sequences. Using a combination of theory and time-resolved optical reflectivity measurements, we report evidence of such order parameter reversal in Ta$_2$NiSe$_5$ based on the anomalous behavior of its coherently excited order-parameter-coupled phonons. Our work expands the field of ultrafast order parameter control beyond spin and charge ordered materials.
Comments: 6 pages main text, 4 figures, 8 pages supplementary information
Subjects: Strongly Correlated Electrons (cond-mat.str-el); Materials Science (cond-mat.mtrl-sci)
Journal reference: Phys. Rev. Lett. 125, 267602 (2020)
DOI: 10.1103/PhysRevLett.125.267602
Cite as: arXiv:2012.12912 [cond-mat.str-el]
  (or arXiv:2012.12912v1 [cond-mat.str-el] for this version)

Submission history

From: David Hsieh [view email]
[v1] Wed, 23 Dec 2020 19:00:45 GMT (8649kb,D)

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