Title: Power-dependent destabilization forces in trapping nanographene-based nanoparticles

Abstract: In recent years, plasmonic optical tweezers have been used to trap nanoparticles and study interactions with their environment. An unavoidable challenge is the plasmonic heating due to resonant excitation and the resulting temperature rise in the surrounding environment. In this work, we demonstrate optical trapping of nanographene-based polymeric nanoparticles using metamaterial plasmonic tweezers. We achieved superior trapping performance and trap stiffness values as high as 8.8 (fN/nm)/(mW/$\mu\mbox{m}^2$) with optical intensities lower than 1 (mW/$\mu\mbox{m}^2$). A range of incident intensities was used to monitor the effect of increasing intensity in the trapping performance. Higher intensities resulted in stronger optical forces, but thermal effects tended to destabilize the trapping. Beyond a critical intensity, where the temperature rise reached 24$^o$C, a large number of particles were being trapped with lower stiffness values indicating the presence of thermal flows. We, therefore, identified a safe intensity regime to avoid detrimental thermal effects. Our platform is ideal for multiple particle trapping in an array configuration and could be used for stable nanopositioning of quantum emitters with controlled interactions with their environment, potentially useful in the field of quantum technologies.